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Vinyl figures for the most part can be modified with polyclay. But some of the stiffer vinyls have some filler in them that distorts with heat. Urethane and styrene figures cannot safely be baked. Epoxy putty of some sort is the general answer. There are a lot of epoxy putties available and it's worth testing a few to find one that you feel comfortable with. There are other build-up materials such as Acrylic gel that also work well with most vinyl figures.
Chris
 
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